Biosynthesis of the benzoyl moiety of cocaine from cinnamic acid via (R)-(+)-3-hydroxy-3-phenylpropanoic acid

Phytochemistry
1992.0

Abstract

trans-[3-C-13,C-14]Cinnamic acid and the N-acetylcysteamine thioester of [3-C-13,C-14]-trans-cinnamic acid served as precursors of the benzoyl moiety of cocaine when fed to intact Erythroxylum coca plants. The specific incorporation of the thioester into the benzoyl carbonyl group of cocaine was established by means of C-13 NMR spectroscopy. (R)-(+)-[3-C-14]-3-hydroxy-3-phenylpropanoic acid was 11 times more effective than its (S)-(-)-isomer as a precursor of the benzoyl moiety of cocaine. A chemical degradation of the cocaine indicated that all the C-14 was located on its benzoyl moiety. Thus, the stereochemistry of the hydroxy group in 3-hydroxy-3-phenylpropanoic acid, is the same as that in the coenzyme A esters of 3-hydroxy fatty acids which are intermediates in the beta-oxidation of fatty acids.

Knowledge Graph

Similar Paper

Biosynthesis of the benzoyl moiety of cocaine from cinnamic acid via (R)-(+)-3-hydroxy-3-phenylpropanoic acid
Phytochemistry 1992.0
Hydroxycinnamic acid esters of isocitric acid: Accumulation and enzymatic synthesis in Amaranthus cruentus
Phytochemistry 1987.0
Lesser alkaloids of cocaine-bearing plants II. 3-Oxo-substituted tropane esters: detection and mass spectral characterization of minor alkaloids found in South American Erythroxylum coca var. coca
Journal of Chromatography A 1996.0
Stereospecificity of the enzymic dehydrogenation in the biosynthesis of 3-ethylidene-L-azetidine-2-carboxylic acid from isoleucine by Streptomyces cacaoi
Biochemistry 1981.0
Lesser alkaloids of cocaine-bearing plants III. 2-carbomethoxy-3-oxo substituted tropane esters: detection and gas chromatographic-mass spectrometric characterization of new minor alkaloids found in South American Erythroxylum coca var. coca
Journal of Chromatography A 1996.0
A Plant-like Biosynthesis of Benzoyl-CoA in the Marine Bacterium ‘Streptomyces maritimus’
Tetrahedron 2000.0
Discovery and Engineering of the Cocaine Biosynthetic Pathway
Journal of the American Chemical Society 2022.0
Synthesis and biological activity of cocaine analogs. 2. 6H-[2]Benzopyrano[4,3-c]pyridin-6-ones
Journal of Medicinal Chemistry 1979.0
Biosynthesis of lathyrine in lathyrus tingitanus
Phytochemistry 1973.0
Nuclear Magnetic Resonance and Biosynthetic Studies of Neoantimycin and Structure Elucidation of Isoneoantimycin, a Minor Metabolite Related to Neoantimycin
Journal of Natural Products 1998.0