Aldgamycin G, a new macrolide antibiotic.

The Journal of Antibiotics
1986.0

Abstract

During the course of screening for new antimicrobial antibiotics, the cultured broth of microorganism No. 1117 (identified as Streptomyces avidinii, isolated from a soil sample collected in Ikeda, Hokkaido, Japan) showed marked antimicrobial activity against Gram-positive bacteria and was found to contain a new macrolide antibiotic named aldgamycin G (1) together with aldgamycin F (2). This communication reports the isolation and characterization of aldgamycin G and F. The organism was cultured at 27°C for 48 hours in a 300-liter fermentation tank. The culture filtrate was processed via Diaion HP-20 column chromatography, followed by silica gel column chromatography and Toyoparl HW 40F column chromatography, yielding pure aldgamycin G (1, 77 mg) and aldgamycin F (2, 43 mg). Physico-chemical properties of 1 and 2 are shown in Table 1. The 13C NMR spectra (Table 2), mass spectrometry, and COSY/NOESY spectra indicated that aldgamycin G (1) is an 8-dehydroxy derivative of aldgamycin F (2). Antimicrobial activity (Table 3) showed that aldgamycin G (1) exhibited higher activity against Gram-positive bacteria than aldgamycin F (2), with MICs comparable to or better than josamycin against strains like Staphylococcus aureus Smith and Bacillus cereus IAM1729. In vivo chemotherapeutic activity (Table 4) revealed that aldgamycin G (1) had an ED50 of 0.6 mg/mouse against S. aureus Smith-infected mice, superior to josamycin (1.2 mg/mouse) and erythromycin (1.0 mg/mouse), though it was less effective against some clinically isolated strains such as Streptococcus pyogenes DP type 2.

Knowledge Graph

Similar Paper