Caprazamycin B, a Novel Anti-tuberculosis Antibiotic, from Streptomyces sp.

The Journal of Antibiotics
2003.0

Abstract

Tuberculosis is still the greatest single infectious cause of mortality in the world. Moreover, the spread of HIV has increased the number of tuberculosis patients, yet powerful new anti-TB drugs with new mechanisms of action have not been developed in over thirty years, with only first-line antituberculous drugs still in use. We screened for new antimycobacterial antibiotics from microbial products with effective and specific narrow-range spectra, and as part of this program, discovered a novel anti-tuberculosis antibiotic named caprazamycin B (CPZ-B) from the culture broth of the Actinomycete strain Streptomyces sp. MK730-62F2. CPZ-B is a new lipo-nucleoside antibiotic related to liposidomycins and capuramycin, with a molecular formula of C53H86N5O22. It showed excellent in vitro anti-mycobacterial activity against drug-susceptible and multidrug-resistant M. tuberculosis strains: MICs were 3.13 μg/ml for M. tuberculosis H37Rv and Kurono strains, 3.13 μg/ml for M. bovis Ravenel strain, 6.25–12.5 μg/ml for drug-susceptible M. tuberculosis (n=22), and 6.25–12.5 μg/ml for multidrug-resistant M. tuberculosis (n=12). It also exhibited in vitro activity equivalent to clarithromycin against Mycobacterium avium complex (MAC), with MICs of 6.25–50 μg/ml for M. avium (n=33) and 1.56–25 μg/ml for M. intracellulare (n=17). CPZ-B demonstrated no significant toxicity in mice (single dose >200 mg/kg i.v., repeated dose 100 mg/kg for 14 days) and no genotoxicity or cytotoxicity (5000 μg/ml). Thus, CPZ-B is considered a promising candidate for an anti-TB drug.

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