Occurrence of gonyautoxin-8 and its epimer in toxic plankton Protogonyaulax tamarensis from Funka Bay, Hokkaido.

Eisei kagaku
1984.0

Abstract

The components of paralytic shellfish poisons produced by toxic plankton Protogonyaulax tamarensis from Funka Bay, Hokkaido, were investigated.The cells of P. tamarensis cultured in BSW-4 medium were extracted with 80% ethanol (pH 2.0). The extract was defatted with chloroform, and then purified by two types of column chromatography on Bio-Gel P-2 and Bio-Rex 70 (H+). The toxins thus obtained were analyzed by using cellulose acetate membrane electrophoresis and thin layer chromatography on silica-gel.From the toxic fractions unbound on Bio-Rex 70 column, four components coded tentatively as PTX₁, PTX₂, PTX₃ and PTX₄ were detected. Judging from Rm values, Rf values and the result of acid-hydrolysis, PTX₁ and PTX₂ were demonstrated to be gonyautoxin-8 and its epimer, respectively. On the other hand, from the toxic fractions bound on Bio-Rex 70 column, gonyautoxins 1-4, neosaxitoxin and saxitoxin were detected.

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