The isolation of cephaeline, emetine, psychotrine(2), tubulesine(3-5), desmethyltubulosine (6,7) and iso-tubulosine (8) have already been reported from the root-bark of Alangium lamarchii Thw. (Alangiaceae). We now report two more new phenolic alkaloids designated as desmethylpsychotrine, m.p. 166-168°, √aJ_n + 67.9° ( e 0.50 MeOH ) and alangioine, m.p. 147-148°, √α]_n + 64.1° ( ⊚ 0.26 MeOH ) from the same seurce.