Extracellularly oxidative activation and inactivation of matured prodrug for cryptic self-resistance in naphthyridinomycin biosynthesis

Proceedings of the National Academy of Sciences
2018.0

Abstract

<jats:title>Significance</jats:title> <jats:p>The shielding strategy for self-resistance in antibiotic biosynthesis from bacteria has been known to employ reversible group-transfer reactions that usually do not directly act on the antibiotic pharmacophore. Typically, the phosphorylation-modified, glycosylation-modified, acetylation-modified, and prepeptide-modified prodrug need to be activated by removing the protection group during or following export and, thereby, employing the hydrolysis reaction as the final step. Herein, we discover an unprecedented oxidative activation and overoxidative inactivation of a matured prodrug; significantly, the oxidation reaction directly deals with the drug warhead and occurs outside the host cells. This cryptic self-resistance mechanism sheds light on antibiotic resistance and the complex biology of extracellular environment.

Knowledge Graph

Similar Paper

Extracellularly oxidative activation and inactivation of matured prodrug for cryptic self-resistance in naphthyridinomycin biosynthesis
Proceedings of the National Academy of Sciences 2018.0
Exploitation of Antibiotic Resistance as a Novel Drug Target: Development of a β-Lactamase-Activated Antibacterial Prodrug
Journal of Medicinal Chemistry 2019.0
Modification of existing antibiotics in the form of precursor prodrugs that can be subsequently activated by nitroreductases of the target pathogen
Bioorganic &amp; Medicinal Chemistry Letters 2016.0
Studies on prodrugs. 11. Synthesis and antimicrobial activity of N-[(4-methyl-5-methylene-2-oxo-1,3-dioxolan-4-yl)oxy]norfloxacin
Journal of Medicinal Chemistry 1989.0
A Two-Step Mechanism for the Activation of Actinorhodin Export and Resistance in Streptomyces coelicolor
mBio 2012.0
Puromycin A, B and C, cryptic nucleosides identified from Streptomyces alboniger NRRL B-1832 by PPtase-based activation
Synthetic and Systems Biotechnology 2018.0
<i>In Situ</i> Activation and Heterologous Production of a Cryptic Lantibiotic from an African Plant Ant-Derived <i>Saccharopolyspora</i> Species
Applied and Environmental Microbiology 2020.0
Activation of a silent phenazine biosynthetic gene cluster reveals a novel natural product and a new resistance mechanism against phenazines
MedChemComm 2012.0
Development of dual-acting prodrugs for circumventing multidrug resistance
Bioorganic &amp; Medicinal Chemistry Letters 2009.0
Genome mining and homologous comparison strategy for digging exporters contributing self-resistance in natamycin-producing Streptomyces strains
Applied Microbiology and Biotechnology 2020.0