Five Additional Genes Are Involved in Clavulanic Acid Biosynthesis in Streptomyces clavuligerus

Antimicrobial Agents and Chemotherapy
2004.0

Abstract

<jats:title>ABSTRACT</jats:title> <jats:p> An approximately 12.5-kbp region of DNA sequence from beyond the end of the previously described clavulanic acid gene cluster was analyzed and found to encode nine possible open reading frames (ORFs). Involvement of these ORFs in clavulanic acid biosynthesis was assessed by creating mutants with defects in each of the ORFs <jats:italic>. orf12</jats:italic> and <jats:italic>orf14</jats:italic> had been previously reported to be involved in clavulanic acid biosynthesis. Now five additional ORFs are shown to play a role, since their mutation results in a significant decrease or total absence of clavulanic acid production. Most of these newly described ORFs encode proteins with little similarity to others in the databases, and so their roles in clavulanic acid biosynthesis are unclear. Mutation of two of the ORFs, <jats:italic>orf15</jats:italic> and <jats:italic>orf16</jats:italic> , results in the accumulation of a new metabolite, <jats:italic>N</jats:italic> -acetylglycylclavaminic acid, in place of clavulanic acid. <jats:italic>orf18</jats:italic> and <jats:italic>orf19</jats:italic> encode apparent penicillin binding proteins, and while mutations in these genes have minimal effects on clavulanic acid production, their normal roles as cell wall biosynthetic enzymes and as targets for β-lactam antibiotics, together with their clustered location, suggest that they are part of the clavulanic acid gene cluster.

Knowledge Graph

Similar Paper

Five Additional Genes Are Involved in Clavulanic Acid Biosynthesis in <i>Streptomyces clavuligerus</i>
Antimicrobial Agents and Chemotherapy 2004.0
Expansion of the Clavulanic Acid Gene Cluster: Identification and In Vivo Functional Analysis of Three New Genes Required for Biosynthesis of Clavulanic Acid by <i>Streptomyces clavuligerus</i>
Journal of Bacteriology 2000.0
Enzymes Catalyzing the Early Steps of Clavulanic Acid Biosynthesis Are Encoded by Two Sets of Paralogous Genes in <i>Streptomyces clavuligerus</i>
Antimicrobial Agents and Chemotherapy 2000.0
ORF17 from the Clavulanic Acid Biosynthesis Gene Cluster Catalyzes the ATP-dependent Formation of N-Glycyl-clavaminic Acid
Journal of Biological Chemistry 2006.0
Cloning, sequencing and disruption of a gene from Streptomyces clavuligerus involved in clavulanic acid biosynthesis
Gene 1994.0
Two Sets of Paralogous Genes Encode the Enzymes Involved in the Early Stages of Clavulanic Acid and Clavam Metabolite Biosynthesis in <i>Streptomyces clavuligerus</i>
Antimicrobial Agents and Chemotherapy 2004.0
Genes Specific for the Biosynthesis of Clavam Metabolites Antipodal to Clavulanic Acid Are Clustered with the Gene for Clavaminate Synthase 1 in <i>Streptomyces clavuligerus</i>
Antimicrobial Agents and Chemotherapy 1999.0
Role of σ-factor (orf21) in clavulanic acid production in Streptomyces clavuligerus NRRL3585
Microbiological Research 2011.0
Clavulanic acid biosynthesis and genetic manipulation for its overproduction
Applied Microbiology and Biotechnology 2010.0
Mutants of <i>Streptomyces clavuligerus</i> with Disruptions in Different Genes for Clavulanic Acid Biosynthesis Produce Large Amounts of Holomycin: Possible Cross-Regulation of Two Unrelated Secondary Metabolic Pathways
Journal of Bacteriology 2002.0