A Common Origin for Guanidinobutanoate Starter Units in Antifungal Natural Products

Angewandte Chemie International Edition
2013.0

Abstract

Keeping it basic: Arginine provides the exotic 4-guanidinobutanoate starter unit for two different types of zwitterionic polyketide (an example for one type is shown in the picture) produced by the same Streptomyces bacterium. The three-step precursor pathway is initiated by a remarkable decarboxylating monooxygenase with high specificity for arginine.

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