Exploring Heteroaromatic Rings as a Replacement for the Labile Amide of Antiplasmodial Pantothenamides

Journal of Medicinal Chemistry
2021.0

Abstract

Malaria-causing <i>Plasmodium</i> parasites are developing resistance to antimalarial drugs, providing the impetus for new antiplasmodials. Although pantothenamides show potent antiplasmodial activity, hydrolysis by pantetheinases/vanins present in blood rapidly inactivates them. We herein report the facile synthesis and biological activity of a small library of pantothenamide analogues in which the labile amide group is replaced with a heteroaromatic ring. Several of these analogues display nanomolar antiplasmodial activity against <i>Plasmodium falciparum</i> and/or <i>Plasmodium knowlesi</i>, and are stable in the presence of pantetheinase. Both a known triazole and a novel isoxazole derivative were further characterized and found to possess high selectivity indices, medium or high Caco-2 permeability, and medium or low microsomal clearance <i>in vitro</i>. Although they fail to suppress <i>Plasmodium berghei</i> proliferation <i>in vivo</i>, the pharmacokinetic and contact time data presented provide a benchmark for the compound profile likely required to achieve antiplasmodial activity in mice and should facilitate lead optimization.

Knowledge Graph

Similar Paper

Exploring Heteroaromatic Rings as a Replacement for the Labile Amide of Antiplasmodial Pantothenamides
Journal of Medicinal Chemistry 2021.0
Structure-activity analysis of CJ-15,801 analogues that interact with Plasmodium falciparum pantothenate kinase and inhibit parasite proliferation
European Journal of Medicinal Chemistry 2018.0
Benzoheterocyclic amodiaquine analogues with potent antiplasmodial activity: Synthesis and pharmacological evaluation
Bioorganic &amp; Medicinal Chemistry Letters 2012.0
Synthesis and biological evaluation of adamantane-based aminophenols as a novel class of antiplasmodial agents
Bioorganic &amp; Medicinal Chemistry Letters 2015.0
3-Hydroxy-N′-arylidenepropanehydrazonamides with Halo-Substituted Phenanthrene Scaffolds Cure P. berghei Infected Mice When Administered Perorally
Journal of Medicinal Chemistry 2017.0
Antimalarial benzoheterocyclic 4-aminoquinolines: Structure–activity relationship, in vivo evaluation, mechanistic and bioactivation studies
Bioorganic &amp; Medicinal Chemistry 2015.0
Evaluation of Aminohydantoins as a Novel Class of Antimalarial Agents
ACS Medicinal Chemistry Letters 2014.0
Synthesis of five libraries of 6,5-fused heterocycles to establish the importance of the heterocyclic core for antiplasmodial activity
Bioorganic &amp; Medicinal Chemistry 2018.0
Structure–activity relationship studies of antiplasmodial aminomethylthiazoles
Bioorganic &amp; Medicinal Chemistry Letters 2014.0
Potent antiplasmodial alkaloids from the rhizobacterium Pantoea agglomerans as hemozoin modulators
Bioorganic Chemistry 2021.0