Sparsifol (1), a new stereoisomer of inositol, and proaporphine alkaloid crotsparsidine (2), have been isolated from the EtOH extract of Crown sparsiflorus. Their structures were determined on the basis of H-1 and C-13 NMR spectra, DEPT, COSY, NOESY, HMBC, HMQC, EI-MS, and FAB-MS experiments.