Four new tetrahydroisoquinoline-monoterpene glucosides, trans-cephaeloside, cis-cephaeloside, 6-0 methyl-trans-cephaeloside and 6-0-methyl-cis-cephaeloside, have been isolated from the roots of Cephaelis ipecacuunha. Their structures have been elucidated on the basis of chemical and spectral data.