Preparation and in vitro activity of aryl ether derivatives of the FK-506 related immunosuppressive macrolides ascomycin and L-683,742

Bioorganic & Medicinal Chemistry Letters
1995.0

Abstract

The arylation of the immunosuppressive macrolides ascomycin and L-683,742 using pentavalent bismuth reagents is described. The in vitro activities of the aryl ether analogs are reported. The macrolide FK-506 (1) is a fungal metabolite first isolated and characterized in 1987.1 It has been shown to be a powerful immunosuppressant in vitro and in vivo, 2 being 50 to 100 times more potent than cyclosporin A - the therapy of choice for prevention of graft rejection following organ transplantation. Although structurally dissimilar, FK-506 and cyclosporin have been shown to elicit their immunosuppressive effects through a common mechanism. 3 Specifically, both bind with their cognate receptors (FKBP and cyclophilin, respectively) and those drugreceptor complexes inhibit the Ca2÷-dependent protein phosphatase calcineurin. The inhibition of calcineurin interferes with early gene transcription following T-cell activation and results in suppression of lymphocyte proliferation. More importantly, FK-506, like cyclosporin, has been shown to be effective in the prevention of organ graft rejection in the clinic. 4 Unfortunately, there are side effects associated with the clinical use of FK-506:most notably nephrotoxicity, neurotoxicity and gastric toxicity.4, 5 Research in these laboratories has focused on the derivatization of ascomycin (2) (L-683,590, FK-520) and its 31-desmethyl congener L-683,742 (3), in an effort to identify a less toxic immunosuppressant. This communication is a preliminary account of the synthesis, via novel organobismuth chemistry, and in vitro immunosuppressive activity of a new class of 31- and 32-O-aryl ethers.

Knowledge Graph

Similar Paper

Preparation and in vitro activity of aryl ether derivatives of the FK-506 related immunosuppressive macrolides ascomycin and L-683,742
Bioorganic & Medicinal Chemistry Letters 1995.0
Alkyl ether derivatives of the FK-506 related, immunosuppressive macrolide L-683,742 (C31-O-desmethyl ascomycin)
Bioorganic & Medicinal Chemistry Letters 1994.0
C32-O-imidazol-2-yl-methyl ether derivatives of the immunosuppressant ascomycin with improved therapeutic potential
Bioorganic & Medicinal Chemistry Letters 1998.0
Potent immunosuppressive C32-O-arylethyl ether derivatives of ascomycin with reduced toxicity
Bioorganic & Medicinal Chemistry Letters 1999.0
Alkyl ether analogs of the FK-506 related, immunosuppressive macrolide L-683,590 (ascomycin)
Bioorganic & Medicinal Chemistry Letters 1994.0
Novel derivatives at the C21 position of the FK-506 macrocycle
Bioorganic & Medicinal Chemistry Letters 1993.0
Microbial transformations of immunosuppressive compounds. IV. Hydroxylation and hemiketal formation of ascomycin(immunomycin) by Streptomyces sp. MA6970(ATCC No.55281).
The Journal of Antibiotics 1994.0
Biosynthesis of Nonimmunosuppressive FK506 Analogues with Antifungal Activity
Journal of Natural Products 2019.0
32-Ascomycinyloxyacetic Acid Derived Immunosuppressants. Independence of Immunophilin Binding and Immunosuppressive Potency
Journal of Medicinal Chemistry 1998.0
Studies on an immunosuppressive macrolactam, ascomycin: Synthesis of a C-33 hydroxyl derivative
Bioorganic & Medicinal Chemistry Letters 1998.0